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If you create a smart campaign with the smart list being clicks link in email (with the link you would like to unsubscribe someone) and then the flow change data value unsubscribe = true, you should be able to achieve this. :)
I personally would only put this on a Unsubscribe Now link.
But I'd also be reluctant to rely totally on this method because the link could break or not come with the token necessary to identify the lead.